The patent badge is an abbreviated version of the USPTO patent document. The patent badge does contain a link to the full patent document.

The patent badge is an abbreviated version of the USPTO patent document. The patent badge covers the following: Patent number, Date patent was issued, Date patent was filed, Title of the patent, Applicant, Inventor, Assignee, Attorney firm, Primary examiner, Assistant examiner, CPCs, and Abstract. The patent badge does contain a link to the full patent document (in Adobe Acrobat format, aka pdf). To download or print any patent click here.

Date of Patent:
Mar. 27, 2018

Filed:

Sep. 09, 2014
Applicant:

The Board of Trustees of the University of Illinois, Urbana, IL (US);

Inventors:

M. Christina White, Champaign, IL (US);

Paul E. Gormisky, Watertown, MA (US);

Attorneys:
Primary Examiner:
Assistant Examiner:
Int. Cl.
CPC ...
C07F 15/00 (2006.01); B01J 31/18 (2006.01); C07B 33/00 (2006.01); C07C 67/29 (2006.01); C07D 307/93 (2006.01); C07D 493/18 (2006.01); C07F 15/02 (2006.01); G06F 19/00 (2018.01);
U.S. Cl.
CPC ...
B01J 31/184 (2013.01); B01J 31/1815 (2013.01); C07B 33/00 (2013.01); C07C 67/29 (2013.01); C07D 307/93 (2013.01); C07D 493/18 (2013.01); C07F 15/025 (2013.01); G06F 19/702 (2013.01); B01J 2231/70 (2013.01); B01J 2531/0258 (2013.01); B01J 2531/842 (2013.01); Y02P 20/582 (2015.11);
Abstract

The invention provides simple small molecule, non-heme iron catalyst systems with broad substrate scope that can predictably enhance or overturn a substrate's inherent reactivity preference for sp3-hybridized C—H bond oxidation. The invention also provides methods for selective aliphatic C—H bond oxidation. Furthermore, a structure-based catalyst reactivity model is disclosed that quantitatively correlates the innate physical properties of the substrate to the site-selectivities observed as a function of the catalyst. The catalyst systems can be used in combination with oxidants such as hydrogen peroxide to effect highly selective oxidations of unactivated sp3 C—H bonds over a broad range of substrates.


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