The patent badge is an abbreviated version of the USPTO patent document. The patent badge does contain a link to the full patent document.

The patent badge is an abbreviated version of the USPTO patent document. The patent badge covers the following: Patent number, Date patent was issued, Date patent was filed, Title of the patent, Applicant, Inventor, Assignee, Attorney firm, Primary examiner, Assistant examiner, CPCs, and Abstract. The patent badge does contain a link to the full patent document (in Adobe Acrobat format, aka pdf). To download or print any patent click here.

Date of Patent:
Mar. 07, 2017

Filed:

Dec. 12, 2013
Applicant:

California Institute of Technology, Pasadena, CA (US);

Inventors:

Lauren E. Rosebrugh, Pasadena, CA (US);

Myles B. Herbert, Somerville, MA (US);

Vanessa M. Marx, Los Angeles, CA (US);

Benjamin K. Keitz, San Francisco, CA (US);

Robert H. Grubbs, South Pasadena, CA (US);

Assignee:
Attorney:
Primary Examiner:
Int. Cl.
CPC ...
C07F 15/00 (2006.01); B01J 31/22 (2006.01); C08G 61/08 (2006.01); C07C 2/34 (2006.01); C07C 29/00 (2006.01); C07C 45/67 (2006.01); C07C 67/293 (2006.01); C07D 313/00 (2006.01); C08F 110/14 (2006.01);
U.S. Cl.
CPC ...
C07F 15/0046 (2013.01); B01J 31/2265 (2013.01); B01J 31/2278 (2013.01); C07C 2/34 (2013.01); C07C 29/00 (2013.01); C07C 45/673 (2013.01); C07C 67/293 (2013.01); C07D 313/00 (2013.01); C08F 110/14 (2013.01); C08G 61/08 (2013.01); B01J 2231/20 (2013.01); B01J 2231/32 (2013.01); B01J 2531/821 (2013.01); C08G 2261/418 (2013.01);
Abstract

A novel chelated ruthenium-based metathesis catalyst bearing an N-2,6-diisopropylphenyl group is reported and displays near-perfect selectivity for the Z-olefin (>95%), as well as unparalleled TONs of up to 7,400, in a variety of homodimerization and industrially relevant metathesis reactions. This derivative and other new catalytically-active species were synthesized using an improved method employing sodium carboxylates to induce the salt metathesis and C—H activation of these chelated complexes. All of these new ruthenium-based catalysts are highly Z-selective in the homodimerization of terminal olefins.


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