The patent badge is an abbreviated version of the USPTO patent document. The patent badge does contain a link to the full patent document.

The patent badge is an abbreviated version of the USPTO patent document. The patent badge covers the following: Patent number, Date patent was issued, Date patent was filed, Title of the patent, Applicant, Inventor, Assignee, Attorney firm, Primary examiner, Assistant examiner, CPCs, and Abstract. The patent badge does contain a link to the full patent document (in Adobe Acrobat format, aka pdf). To download or print any patent click here.

Date of Patent:
Feb. 24, 2015

Filed:

Nov. 18, 2011
Applicants:

Qilin Zhou, Tianjin, CN;

Jianhua Xie, Tianjin, CN;

Xiaoyan Liu, Tianjin, CN;

Jianbo Xie, Tianjin, CN;

Lixin Wang, Tianjin, CN;

Inventors:

Qilin Zhou, Tianjin, CN;

Jianhua Xie, Tianjin, CN;

Xiaoyan Liu, Tianjin, CN;

Jianbo Xie, Tianjin, CN;

Lixin Wang, Tianjin, CN;

Attorney:
Primary Examiner:
Int. Cl.
CPC ...
C07F 9/06 (2006.01); B01J 31/24 (2006.01); B01J 31/18 (2006.01); C07B 53/00 (2006.01); C07C 29/145 (2006.01); C07C 41/26 (2006.01); C07C 67/31 (2006.01); C07D 307/83 (2006.01); C07F 9/58 (2006.01); C07F 9/60 (2006.01); C07B 41/02 (2006.01); C07F 15/00 (2006.01);
U.S. Cl.
CPC ...
B01J 31/249 (2013.01); B01J 31/189 (2013.01); C07B 53/00 (2013.01); C07C 29/145 (2013.01); C07C 41/26 (2013.01); C07C 67/31 (2013.01); C07D 307/83 (2013.01); C07F 9/588 (2013.01); C07F 9/60 (2013.01); C07B 41/02 (2013.01); C07F 15/004 (2013.01); B01J 2231/643 (2013.01); B01J 2531/827 (2013.01); C07B 2200/07 (2013.01); C07C 2101/14 (2013.01); C07C 2102/08 (2013.01); C07C 2102/10 (2013.01);
Abstract

The present invention relates to a chiral spiro-pyridylamidophosphine ligand compound, synthesis method therefor and application thereof. The chiral spiro-pyridylamidophosphine compound is a compound having a structure of Formula (I), a racemate or optical isomer thereof, or a catalytically acceptable salt thereof, and is mainly characterized by having a chiral spiro-dihydro-indene skeleton in its structure. The chiral spiro-pyridylamidophosphine compound may be synthesized with optical active 7-diaryl/alkylphosphino-7'-amino-1,1′-spiro-dihydro-indene or substituted 7-diaryl/alkylphosphino-7′-amino-1,1′-spiro-dihydro-indene having a spiro-skeleton as chiral starting material. The chiral spiro-pyridylamidophosphine compound may be used as a chiral ligand in asymmetric hydrogenation of a carbonyl compound catalyzed by iridium, in which the reaction activity is very high, the amount of the catalyst may be 0.0001 mol %, and the enantioselectivity of the reaction is up to 99.9% ee.


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