The patent badge is an abbreviated version of the USPTO patent document. The patent badge does contain a link to the full patent document.

The patent badge is an abbreviated version of the USPTO patent document. The patent badge covers the following: Patent number, Date patent was issued, Date patent was filed, Title of the patent, Applicant, Inventor, Assignee, Attorney firm, Primary examiner, Assistant examiner, CPCs, and Abstract. The patent badge does contain a link to the full patent document (in Adobe Acrobat format, aka pdf). To download or print any patent click here.

Date of Patent:
Oct. 10, 2017

Filed:

Apr. 15, 2016
Applicant:

Lucite International Uk Limited, Southampton, Hampshire, GB;

Inventors:

Sabina Ziemian, Wilton, GB;

Ian Andrew York, Wilton, GB;

Assignee:
Attorney:
Primary Examiner:
Int. Cl.
CPC ...
B01J 27/18 (2006.01); C07C 67/343 (2006.01); B01J 37/03 (2006.01); B01J 23/04 (2006.01); B01J 35/00 (2006.01); B01J 35/10 (2006.01); B01J 27/182 (2006.01); B01J 35/02 (2006.01); C07C 67/30 (2006.01); B01J 23/02 (2006.01); B01J 23/10 (2006.01);
U.S. Cl.
CPC ...
B01J 27/1806 (2013.01); B01J 23/04 (2013.01); B01J 27/18 (2013.01); B01J 27/182 (2013.01); B01J 35/002 (2013.01); B01J 35/02 (2013.01); B01J 35/1009 (2013.01); B01J 35/1014 (2013.01); B01J 37/03 (2013.01); C07C 67/30 (2013.01); C07C 67/343 (2013.01); B01J 23/02 (2013.01); B01J 23/10 (2013.01);
Abstract

A method of producing an ethylenically unsaturated carboxylic acid or ester such as (meth) acrylic acid or alkyl esters thereof, for example, methyl methacrylate is described. The process comprises the steps of contacting formaldehyde or a suitable source thereof with a carboxylic acid or ester, for example, propionic acid or alkyl esters thereof in the presence of a catalyst and optionally an alcohol. The catalyst comprises group II metal phosphate crystals having rod or needle like morphology or a suitable source thereof. The phosphate may be a hydroxyapatite, pyrophosphate, hydroxyphosphate, POphosphate or mixtures thereof. The group II metal may be selected from Ca, Sr, Ba or mixtures thereof, for example, strontium hydroxyapatite and calcium hydroxyapatite. A catalyst system comprising a crystalline metal phosphate catalyst and a catalyst support is also described. The metal phosphate has rod/needle like morphology.


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