The patent badge is an abbreviated version of the USPTO patent document. The patent badge does contain a link to the full patent document.

The patent badge is an abbreviated version of the USPTO patent document. The patent badge covers the following: Patent number, Date patent was issued, Date patent was filed, Title of the patent, Applicant, Inventor, Assignee, Attorney firm, Primary examiner, Assistant examiner, CPCs, and Abstract. The patent badge does contain a link to the full patent document (in Adobe Acrobat format, aka pdf). To download or print any patent click here.

Date of Patent:
May. 23, 2017

Filed:

May. 28, 2014
Applicant:

Shanghai Research Institute of Chemical Industry, Shanghai, CN;

Inventors:

An Shen, Shanghai, CN;

Yucai Cao, Shanghai, CN;

Xiangyang Wu, Shanghai, CN;

Xiaofeng Ye, Shanghai, CN;

Chen Ni, Shanghai, CN;

Yongqing Li, Shanghai, CN;

Attorney:
Primary Examiner:
Assistant Examiner:
Int. Cl.
CPC ...
B01J 31/08 (2006.01); B01J 31/10 (2006.01); B01J 35/08 (2006.01); B01J 21/18 (2006.01); C07C 201/14 (2006.01); C07D 301/12 (2006.01); C01B 31/02 (2006.01); B01J 31/22 (2006.01); B01J 31/28 (2006.01); C07C 67/343 (2006.01); C07D 333/16 (2006.01); C07C 45/68 (2006.01); C07C 49/67 (2006.01); C07C 49/784 (2006.01); C07D 295/096 (2006.01); C07D 307/36 (2006.01); C07F 15/00 (2006.01); C07C 209/10 (2006.01); C07C 1/26 (2006.01); C07C 1/32 (2006.01); C07C 213/08 (2006.01); C07D 213/16 (2006.01); C07D 265/30 (2006.01); C07D 333/10 (2006.01);
U.S. Cl.
CPC ...
B01J 31/2273 (2013.01); B01J 31/28 (2013.01); C07C 1/26 (2013.01); C07C 1/321 (2013.01); C07C 1/325 (2013.01); C07C 1/326 (2013.01); C07C 45/68 (2013.01); C07C 49/67 (2013.01); C07C 49/784 (2013.01); C07C 67/343 (2013.01); C07C 209/10 (2013.01); C07C 213/08 (2013.01); C07D 213/16 (2013.01); C07D 265/30 (2013.01); C07D 295/096 (2013.01); C07D 307/36 (2013.01); C07D 333/10 (2013.01); C07D 333/16 (2013.01); C07F 15/006 (2013.01); B01J 2231/4205 (2013.01); B01J 2531/824 (2013.01); C07C 2101/14 (2013.01); C07C 2531/22 (2013.01);
Abstract

The present invention relates to an n-heterocyclic carbene (NHC) type palladium catalyst and its preparation method as well as applications. Its preparation process is as below: select glyoxal as the raw material to synthesize glyoxaldiimine in the presence of Lewis acid or Bronsted acid, and then react with paraformaldehyde to get the NHC type ligand. Use palladiumto react with the compound containing carbon-nitrogen double bonds to get palladiumcyclic dimer; make the palladium cyclic dimer and the NHC type ligand coordinated to get the NHC type palladium catalyst. The palladium catalyst with a brand new structure according to the present invention, boasts high activity and multi-purpose. In addition, it shows excellent reaction activity in a lot of catalytic-coupling reactions including Suzuki-Miyaura, Heck, Buchwald-Hartwig, Kumada-Tamao-Corriu, Sonogashira, Negishi and α-ketone arylation reactions, and some reactions even can be carried out with the presence of an extremely low concentration of catalyst, exhibiting favorable industrialization prospect.


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