The patent badge is an abbreviated version of the USPTO patent document. The patent badge does contain a link to the full patent document.

The patent badge is an abbreviated version of the USPTO patent document. The patent badge covers the following: Patent number, Date patent was issued, Date patent was filed, Title of the patent, Applicant, Inventor, Assignee, Attorney firm, Primary examiner, Assistant examiner, CPCs, and Abstract. The patent badge does contain a link to the full patent document (in Adobe Acrobat format, aka pdf). To download or print any patent click here.

Date of Patent:
Sep. 01, 2015

Filed:

Dec. 13, 2012
Applicant:

Nanyang Technological University, Singapore, SG;

Inventors:

Yonggui Chi, Singapore, SG;

Bhoopendra Tiwari, Singapore, SG;

Assignee:
Attorney:
Primary Examiner:
Int. Cl.
CPC ...
C07C 211/00 (2006.01); C07C 205/00 (2006.01); C07C 207/00 (2006.01); C07C 221/00 (2006.01); C07C 201/12 (2006.01); C07C 205/02 (2006.01); C07C 205/44 (2006.01); C07B 41/06 (2006.01); C07C 225/14 (2006.01); C07C 225/16 (2006.01);
U.S. Cl.
CPC ...
C07C 221/00 (2013.01); C07B 41/06 (2013.01); C07C 201/12 (2013.01); C07C 205/02 (2013.01); C07C 205/44 (2013.01); C07C 225/14 (2013.01); C07C 225/16 (2013.01);
Abstract

Present invention relates to a method of preparing a chiral α- or β-substituted ketone from the corresponding β- or γ-substituted aldehyde, wherein the ketone has formula (I), (III) or (V), and the corresponding aldehyde has formula (II), (IV) or (VI), respectively, the method comprising reacting the aldehyde of formula (II), (IV) or (VI) in the presence of an amine, oxygen and an organic solvent, wherein the reaction is carried out in the absence of a metal-based catalyst or a metal-based oxidant, wherein: R is H, a substituted or unsubstituted C-Calkyl, substituted or unsubstituted C-Calkenyl, substituted or unsubstituted C-Calkynyl, substituted or unsubstituted C-Ccycloalkyl, substituted or unsubstituted C-Ccycloalkenyl, substituted or unsubstituted C-Cheterocycloalkyl, substituted or unsubstituted C-Cheterocycloalkenyl, substituted or unsubstituted C-Caryl, or substituted or unsubstituted C-Cheteroaryl; and R' is H, a substituted or unsubstituted C-Calkyl, substituted or unsubstituted C-Calkenyl, substituted or unsubstituted C-Calkynyl, substituted or unsubstituted C-Ccycloalkyl, substituted or unsubstituted C-Ccycloalkenyl, substituted or unsubstituted C-Cheterocycloalkyl, substituted or unsubstituted C-Cheterocycloalkenyl, substituted or unsubstituted C-Caryl, or substituted or unsubstituted C-Cheteroaryl.


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