The patent badge is an abbreviated version of the USPTO patent document. The patent badge does contain a link to the full patent document.

The patent badge is an abbreviated version of the USPTO patent document. The patent badge covers the following: Patent number, Date patent was issued, Date patent was filed, Title of the patent, Applicant, Inventor, Assignee, Attorney firm, Primary examiner, Assistant examiner, CPCs, and Abstract. The patent badge does contain a link to the full patent document (in Adobe Acrobat format, aka pdf). To download or print any patent click here.

Date of Patent:
Apr. 14, 2015

Filed:

Feb. 18, 2010
Applicants:

Radoslav Adzic, East Setauket, NY (US);

Junliang Zhang, Rochester, NY (US);

Yibo MO, Naperville, IL (US);

Miomir Vukmirovic, Port Jefferson Station, NY (US);

Inventors:

Radoslav Adzic, East Setauket, NY (US);

Junliang Zhang, Rochester, NY (US);

Yibo Mo, Naperville, IL (US);

Miomir Vukmirovic, Port Jefferson Station, NY (US);

Assignee:
Attorneys:
Primary Examiner:
Assistant Examiner:
Int. Cl.
CPC ...
B01J 23/44 (2006.01); H01M 4/92 (2006.01); B82Y 30/00 (2011.01); H01M 4/86 (2006.01); B01J 35/00 (2006.01); H01M 8/10 (2006.01);
U.S. Cl.
CPC ...
H01M 4/921 (2013.01); B01J 23/44 (2013.01); B01J 35/0013 (2013.01); B82Y 30/00 (2013.01); H01M 4/8657 (2013.01); H01M 4/926 (2013.01); H01M 4/928 (2013.01); H01M 2008/1095 (2013.01); Y02E 60/50 (2013.01);
Abstract

Core-shell particles encapsulated by a thin film of a catalytically active metal are described. The particles are preferably nanoparticles comprising a non-noble core with a noble metal shell which preferably do not include Pt. The non-noble metal-noble metal core-shell nanoparticles are encapsulated by a catalytically active metal which is preferably Pt. The core-shell nanoparticles are preferably formed by prolonged elevated-temperature annealing of nanoparticle alloys in an inert environment. This causes the noble metal component to surface segregate and form an atomically thin shell. The Pt overlayer is formed by a process involving the underpotential deposition of a monolayer of a non-noble metal followed by immersion in a solution comprising a Pt salt. A thin Pt layer forms via the galvanic displacement of non-noble surface atoms by more noble Pt atoms in the salt. The overall process is a robust and cost-efficient method for forming Pt-coated non-noble metal-noble metal core-shell nanoparticles.


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