The patent badge is an abbreviated version of the USPTO patent document. The patent badge does contain a link to the full patent document.

The patent badge is an abbreviated version of the USPTO patent document. The patent badge covers the following: Patent number, Date patent was issued, Date patent was filed, Title of the patent, Applicant, Inventor, Assignee, Attorney firm, Primary examiner, Assistant examiner, CPCs, and Abstract. The patent badge does contain a link to the full patent document (in Adobe Acrobat format, aka pdf). To download or print any patent click here.

Date of Patent:
Oct. 28, 2014

Filed:

Apr. 13, 2011
Applicants:

Juntao Liu, Shanghai, CN;

Fengxia Sun, Shanghai, CN;

Jun Kuai, Shanghai, CN;

Inventors:

Juntao Liu, Shanghai, CN;

Fengxia Sun, Shanghai, CN;

Jun Kuai, Shanghai, CN;

Attorneys:
Primary Examiner:
Assistant Examiner:
Int. Cl.
CPC ...
C07C 67/18 (2006.01); C07C 67/36 (2006.01); B01J 23/89 (2006.01); B01J 23/656 (2006.01); B01J 21/04 (2006.01); B01J 21/06 (2006.01);
U.S. Cl.
CPC ...
C07C 67/18 (2013.01); B01J 21/04 (2013.01); B01J 21/063 (2013.01); C07C 67/36 (2013.01); B01J 23/8973 (2013.01); B01J 23/8926 (2013.01); B01J 23/8946 (2013.01); B01J 23/6562 (2013.01); B01J 23/894 (2013.01);
Abstract

The present invention relates to a process of producing oxalate by CO gas phase method for chiefly solving the technical problem of the low utilization efficiency of nitrogen oxides or nitrous acid esters in the prior art. The present invention solves the problem in a better way by using the following steps including: a gas phase stream V containing NO and methanol and oxygen enter a supergravity rotating bed reactor II and are subjected to the oxidative esterification reaction to produce an effluent VI containing methyl nitrite; a methyl nitrite effluent VII obtained from separating said effluent VI together with a CO gas II enter a coupling reactor II and is contacted with a catalyst II to react to form a dimethyl oxalate effluent VIII and a gas phase effluent IX containing NO; the resultant dimethyl oxalate effluent VIII is separated to obtain a dimethyl oxalate product I; optionally, the gas phase effluent IX containing NO is returned to the step above so as to be mixed with the gas phase stream V containing NO for being recycled. Therefore, the process is applicable to the industrial production of oxalate by CO gas phase method.


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