The patent badge is an abbreviated version of the USPTO patent document. The patent badge does contain a link to the full patent document.

The patent badge is an abbreviated version of the USPTO patent document. The patent badge covers the following: Patent number, Date patent was issued, Date patent was filed, Title of the patent, Applicant, Inventor, Assignee, Attorney firm, Primary examiner, Assistant examiner, CPCs, and Abstract. The patent badge does contain a link to the full patent document (in Adobe Acrobat format, aka pdf). To download or print any patent click here.

Date of Patent:
Mar. 07, 2000

Filed:

Apr. 18, 1997
Applicant:
Inventors:

XiaoGuang Yang, Los Alamos, NM (US);

Basil I Swanson, Los Alamos, NM (US);

DeQuan Li, Los Alamos, NM (US);

Assignee:
Attorney:
Primary Examiner:
Int. Cl.
CPC ...
G02F / ; G02F / ;
U.S. Cl.
CPC ...
428333 ; 252582 ; 359328 ; 359329 ; 359330 ; 359332 ; 385122 ; 385129 ; 385130 ; 385131 ; 428405 ; 428429 ; 428447 ; 428451 ;
Abstract

The design and synthesis of a family of calix[4]arene-based nonlinear optical (NLO) chromophores are discussed. The calixarene chromophores are macrocyclic compounds consisting of four simple D-.pi.-A units bridged by methylene groups. These molecules were synthesized such that four D-.pi.-A units of the calix[4]arene were aligned along the same direction with the calixarene in a cone conformation. These nonlinear optical super-chromophores were subsequently fabricated into covalently bound self-assembled monolayers on the surfaces of fused silica and silicon. Spectroscopic second harmonic generation (SHG) measurements were carried out to determine the absolute value of the dominant element of the second-order nonlinear susceptibility, d.sub.33, and the average molecular alignment, .PSI.. A value of d.sub.33 =60 pm/V at a fundamental wavelength of 890 nm, and .PSI..about.36.degree. was found with respect to the surface normal.


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