The patent badge is an abbreviated version of the USPTO patent document. The patent badge does contain a link to the full patent document.

The patent badge is an abbreviated version of the USPTO patent document. The patent badge covers the following: Patent number, Date patent was issued, Date patent was filed, Title of the patent, Applicant, Inventor, Assignee, Attorney firm, Primary examiner, Assistant examiner, CPCs, and Abstract. The patent badge does contain a link to the full patent document (in Adobe Acrobat format, aka pdf). To download or print any patent click here.

Date of Patent:
Oct. 24, 2023

Filed:

Mar. 15, 2021
Applicant:

Soochow University, Suzhou, CN;

Inventors:

Shilei Zhang, Suzhou, CN;

Yujian Mao, Suzhou, CN;

Assignee:

SOOCHOW UNIVERSITY, Suzhou, CN;

Attorney:
Primary Examiner:
Int. Cl.
CPC ...
C07C 45/41 (2006.01); B01J 23/44 (2006.01); B01J 31/12 (2006.01); C07C 49/537 (2006.01); C07C 49/553 (2006.01);
U.S. Cl.
CPC ...
C07C 45/41 (2013.01); B01J 23/44 (2013.01); B01J 31/121 (2013.01); C07C 49/537 (2013.01); C07C 49/553 (2013.01); C07C 2527/10 (2013.01); C07C 2531/12 (2013.01); C07C 2531/30 (2013.01); C07C 2602/08 (2017.05);
Abstract

Provided is an application of a metal hydride/palladium compound system in the preparation of a 1,3-dicarbonyl compound in a cascade reaction of an electron-deficient alkene compound, said reaction comprising the following steps: under the protection of nitrogen, a palladium compound and a metal hydride are suspended and stirred in a solvent, then an electron-deficient alkene compound is added; the mixture reacts at 0° C. to 100° C. for 0.3 to 10 hours; a saturated ammonium chloride aqueous solution is added to stop the reaction, and then extraction, drying by evaporation and purification by column chromatography are performed to obtain the product of 1,3-dicarbonyl compound. The hydride and palladium compound catalysts used in the method are reagents easily obtained in a laboratory; compared with the commonly used methods of hydrogenation with hydrogen gas, the method can be easily operated, and has high safety, mild conditions and high reaction yield.


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