The patent badge is an abbreviated version of the USPTO patent document. The patent badge does contain a link to the full patent document.

The patent badge is an abbreviated version of the USPTO patent document. The patent badge covers the following: Patent number, Date patent was issued, Date patent was filed, Title of the patent, Applicant, Inventor, Assignee, Attorney firm, Primary examiner, Assistant examiner, CPCs, and Abstract. The patent badge does contain a link to the full patent document (in Adobe Acrobat format, aka pdf). To download or print any patent click here.

Date of Patent:
Apr. 18, 2023

Filed:

Mar. 19, 2021
Applicant:

Colorado State University Research Foundation, Fort Collins, CO (US);

Inventors:

Eugene Y. Chen, Fort Collins, CO (US);

Xiaoyan Tang, Fort Collins, CO (US);

Assignee:
Attorneys:
Primary Examiner:
Int. Cl.
CPC ...
C08G 63/08 (2006.01); C08L 67/04 (2006.01); C08G 63/82 (2006.01); B01J 31/22 (2006.01); C08G 63/664 (2006.01);
U.S. Cl.
CPC ...
C08G 63/08 (2013.01); B01J 31/2243 (2013.01); C08G 63/823 (2013.01); C08L 67/04 (2013.01); B01J 2531/0213 (2013.01); B01J 2531/35 (2013.01); B01J 2531/36 (2013.01); C08G 63/664 (2013.01); C08G 2230/00 (2013.01);
Abstract

Biodegradable polymers with advantageous physical and chemical properties are described, as well as methods for making such polymers. In one embodiment, a new chemical synthesis route to technologically important biodegradable poly(3-hydroxybutyrate) (P3HB) with high isotacticity and molecular weight required for a practical use is described. The new route can utilize racemic eight-membered cyclic diolide (rac-DL), meso-DL, or a rac-DL and meso-DL mixture, derived from bio-sourced dimethyl succinate, and enantiomeric (R,R)-DL and (S,S)-DL, optically resolved by metal-based catalysts. With a stereoselective racemic molecular catalyst, the ROP of rac-DL under ambient conditions produces rapidly P3HB with essentially perfect isotacticity ([mm]>99%), high crystallinity and melting temperature (T=171° C.), as well as high molecular weight and low dispersity (M=1.54×10g/mol, Ð=1.01).


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