The patent badge is an abbreviated version of the USPTO patent document. The patent badge does contain a link to the full patent document.

The patent badge is an abbreviated version of the USPTO patent document. The patent badge covers the following: Patent number, Date patent was issued, Date patent was filed, Title of the patent, Applicant, Inventor, Assignee, Attorney firm, Primary examiner, Assistant examiner, CPCs, and Abstract. The patent badge does contain a link to the full patent document (in Adobe Acrobat format, aka pdf). To download or print any patent click here.

Date of Patent:
Sep. 27, 2022

Filed:

Oct. 21, 2019
Applicant:

Nankai University, Tianjin, CN;

Inventors:

Jiangong Ma, Tianjin, CN;

Zhiqiang Wang, Tianjin, CN;

Peng Cheng, Tianjin, CN;

Assignee:

NANKAI UNIVERSITY, Tianjin, CN;

Attorney:
Primary Examiner:
Int. Cl.
CPC ...
C07C 231/12 (2006.01); C07C 51/15 (2006.01); C07C 231/02 (2006.01); C07C 231/14 (2006.01); A01N 37/22 (2006.01); B01J 23/04 (2006.01); B01J 23/72 (2006.01);
U.S. Cl.
CPC ...
C07C 231/12 (2013.01); A01N 37/22 (2013.01); B01J 23/04 (2013.01); B01J 23/72 (2013.01); C07C 51/15 (2013.01); C07C 231/02 (2013.01); C07C 231/14 (2013.01);
Abstract

A process method for producing a pesticide by using carbon dioxide includes: weighing a 1,3-cyclohexanedione substrate 1(a-e), a catalyst and CsCOin a Schlenk bottle, degassing, and continuously introducing 1 atm of carbon dioxide; adding a solvent and reacting for 48 h in an oil bath at 50° C. After the reaction was completed, post-treatment was carried out to obtain a 2-carboxyl-1,3-cyclohexanedione compound 2(a-e). The obtained acid is acylated and then added dropwise to a dichloromethane solution containing aniline to react for 2 h at room temperature. After the reaction, column chromatography was performed to obtain a pesticide compound 3(a-e). Adding the pesticide compound 3(a-e) into 50% concentrated sulfuric acid and refluxing at 80° C. for 8 hours. Through separation, a pesticide product compound 4(a-e) was obtained. The process method is simple, with low requirements on equipment, wide sources of raw materials, low cost, low toxicity and easy industrial scale-up production.


Find Patent Forward Citations

Loading…