The patent badge is an abbreviated version of the USPTO patent document. The patent badge does contain a link to the full patent document.

The patent badge is an abbreviated version of the USPTO patent document. The patent badge covers the following: Patent number, Date patent was issued, Date patent was filed, Title of the patent, Applicant, Inventor, Assignee, Attorney firm, Primary examiner, Assistant examiner, CPCs, and Abstract. The patent badge does contain a link to the full patent document (in Adobe Acrobat format, aka pdf). To download or print any patent click here.

Date of Patent:
Aug. 09, 2022

Filed:

Dec. 04, 2018
Applicant:

California Institute of Technology, Pasadena, CA (US);

Inventors:

Tonia S. Ahmed, Pasadena, CA (US);

T. Patrick Montgomery, Pasadena, CA (US);

Robert H. Grubbs, Pasadena, CA (US);

Assignee:
Attorney:
Primary Examiner:
Int. Cl.
CPC ...
C07D 313/00 (2006.01); B01J 31/22 (2006.01);
U.S. Cl.
CPC ...
C07D 313/00 (2013.01); B01J 31/226 (2013.01); B01J 31/2208 (2013.01); B01J 31/2273 (2013.01); B01J 2231/546 (2013.01); B01J 2531/821 (2013.01);
Abstract

This invention relates generally to the synthesis of E-macrocycles using stereoretentive ruthenium olefin metathesis catalysts supported by dithioiate ligands. Macrocycles were generated with excellent selectivity (>99% E) and in moderate to high/good yields (47% to 80% yield; 58% to 80% yield) from diene starting materials bearing two E-olefins or bearing one E-olefin and one terminal olefin, A variety of rings were constructed, ranging from 12- to 18-membered macrocycles, including the antibiotic recifeiolide. The invention has utility in the fields of organometallics and organic synthesis.


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