The patent badge is an abbreviated version of the USPTO patent document. The patent badge does contain a link to the full patent document.

The patent badge is an abbreviated version of the USPTO patent document. The patent badge covers the following: Patent number, Date patent was issued, Date patent was filed, Title of the patent, Applicant, Inventor, Assignee, Attorney firm, Primary examiner, Assistant examiner, CPCs, and Abstract. The patent badge does contain a link to the full patent document (in Adobe Acrobat format, aka pdf). To download or print any patent click here.

Date of Patent:
Aug. 31, 2021

Filed:

Dec. 20, 2017
Applicant:

Dalian Institute of Chemical Physics, Chinese Academy of Sciences, Dalian, CN;

Inventors:

Bin Liu, Dalian, CN;

Hongbin Yang, Dalian, CN;

Yanqiang Huang, Dalian, CN;

Song Liu, Dalian, CN;

Tao Zhang, Dalian, CN;

Attorney:
Primary Examiner:
Int. Cl.
CPC ...
C25B 11/044 (2021.01); C01B 32/184 (2017.01); B01J 37/08 (2006.01); B01J 35/00 (2006.01); C01B 32/194 (2017.01); C01B 32/40 (2017.01); B01J 23/755 (2006.01); B01J 23/745 (2006.01); C25B 1/00 (2021.01); H01M 4/90 (2006.01); C25B 11/031 (2021.01);
U.S. Cl.
CPC ...
C25B 11/044 (2021.01); B01J 23/745 (2013.01); B01J 23/755 (2013.01); B01J 35/002 (2013.01); B01J 35/0033 (2013.01); B01J 37/086 (2013.01); C01B 32/184 (2017.08); C01B 32/194 (2017.08); C01B 32/40 (2017.08); C25B 1/00 (2013.01); C25B 11/031 (2021.01); H01M 4/90 (2013.01); C01B 2204/22 (2013.01); C01P 2002/52 (2013.01); C01P 2002/72 (2013.01); C01P 2002/85 (2013.01); C01P 2002/86 (2013.01); C01P 2004/03 (2013.01); C01P 2004/04 (2013.01); C01P 2006/40 (2013.01);
Abstract

The present invention relates to a graphene material inlaid with single metal atoms, the preparation method thereof and its application of being used as the catalyst for the electroreduction of carbon dioxide. The graphene material inlaid with single metal atoms comprises single metal atoms and graphene; the single metal atoms are dispersed in the framework of the graphene; and the graphene is at least one selected from N doped graphene and N and S co-doped graphene. The material is used for the electrochemical reduction reaction of carbon dioxide, which significantly improves the utilization efficiency of the metal atoms and enhances the catalytic activity for the electroreduction of carbon dioxide, improves the catalytic stability, inhibits effectively the hydrogen evolution reaction, improves the selectivity for CO product, and broadens the electric potential window of reducing carbon dioxide to generate CO.


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