The patent badge is an abbreviated version of the USPTO patent document. The patent badge does contain a link to the full patent document.

The patent badge is an abbreviated version of the USPTO patent document. The patent badge covers the following: Patent number, Date patent was issued, Date patent was filed, Title of the patent, Applicant, Inventor, Assignee, Attorney firm, Primary examiner, Assistant examiner, CPCs, and Abstract. The patent badge does contain a link to the full patent document (in Adobe Acrobat format, aka pdf). To download or print any patent click here.

Date of Patent:
Jan. 14, 2020

Filed:

Dec. 11, 2015
Applicant:

Dalian Institute of Chemical Physics, Chinese Academy of Sciences, Dalian, CN;

Inventors:

Lei Shi, Dalian, CN;

Youming Ni, Dalian, CN;

Wenliang Zhu, Dalian, CN;

Yong Liu, Dalian, CN;

Hongchao Liu, Dalian, CN;

Zhongmin Liu, Dalian, CN;

Attorneys:
Primary Examiner:
Int. Cl.
CPC ...
C07C 41/14 (2006.01); C07C 29/128 (2006.01); B01J 29/08 (2006.01); B01J 29/18 (2006.01); B01J 29/40 (2006.01); B01J 29/65 (2006.01); B01J 29/78 (2006.01);
U.S. Cl.
CPC ...
C07C 41/14 (2013.01); B01J 29/084 (2013.01); B01J 29/18 (2013.01); B01J 29/40 (2013.01); B01J 29/65 (2013.01); B01J 29/7815 (2013.01); C07C 29/128 (2013.01); Y02P 20/52 (2015.11);
Abstract

The present invention provides a method for directly preparing glycol dimethyl ether and co-producing ethylene glycol from ethylene glycol monomethyl ether. More specifically, the method comprises passing a feedstock containing a raw material of ethylene glycol monomethyl ether and a carrier gas through a reactor loaded with a solid acid catalyst to produce glycol dimethyl ether and ethylene glycol, at a reaction temperature range from 40° C. to 150° C. and a reaction pressure range from 0.1 MPa to 15.0 MPa; wherein a carrier gas is an optional inactive gas; and the feedstock contains water whose volume concentration in the feedstock is in a range from 0% to 95%; and the weight hourly space velocity of the raw material of ethylene glycol monomethyl ether is in a range from 0.05 hto 5.0 h; and the volume concentration of the raw material of ethylene glycol monomethyl ether in the feedstock is in a range from 1% to 100%; and the volume concentration of the carrier gas in the feedstock is in a range from 0% to 99%. In the method of the present invention, using a solid acid as a catalyst and ethylene glycol monomethyl ether as a raw material, under a low temperature condition, glycol dimethyl ether and ethylene glycol are prepared directly with high selectivity; moreover, there is substantially or completely no production of by-product 1,4-dioxane that causes pollution to the environment and is harmful to the human body or animal bodies.


Find Patent Forward Citations

Loading…