The patent badge is an abbreviated version of the USPTO patent document. The patent badge does contain a link to the full patent document.

The patent badge is an abbreviated version of the USPTO patent document. The patent badge covers the following: Patent number, Date patent was issued, Date patent was filed, Title of the patent, Applicant, Inventor, Assignee, Attorney firm, Primary examiner, Assistant examiner, CPCs, and Abstract. The patent badge does contain a link to the full patent document (in Adobe Acrobat format, aka pdf). To download or print any patent click here.

Date of Patent:
Sep. 17, 2019

Filed:

Nov. 10, 2017
Applicant:

The Board of Trustees of the University of Illinois, Urbana, IL (US);

Inventors:

Damien S. Guironnet, Urbana, IL (US);

Michael G. Hyatt, Savoy, IL (US);

Dylan J. Walsh, Sun Prairie, WI (US);

Attorneys:
Primary Examiner:
Int. Cl.
CPC ...
C08K 5/541 (2006.01); C08K 5/54 (2006.01); C08F 10/02 (2006.01); C08F 20/06 (2006.01); C08F 4/80 (2006.01); C08F 110/02 (2006.01); C08F 110/06 (2006.01); C08F 293/00 (2006.01); C08G 81/02 (2006.01); C08G 83/00 (2006.01);
U.S. Cl.
CPC ...
C08K 5/541 (2013.01); C08F 4/80 (2013.01); C08F 10/02 (2013.01); C08F 20/06 (2013.01); C08F 110/02 (2013.01); C08F 110/06 (2013.01); C08F 293/005 (2013.01); C08G 81/027 (2013.01); C08G 83/003 (2013.01); C08G 83/005 (2013.01); C08K 5/5403 (2013.01); C08F 2438/00 (2013.01); C08F 2438/01 (2013.01); C08F 2810/40 (2013.01);
Abstract

A strategy for the synthesis of semi-telechelic polyethylene through the palladium diimine-catalyzed chain transfer polymerization of ethylene using various silanes as chain transfer agents is reported. Polymer molecular weight and end-group chemical structure can be tuned by varying the chain transfer agent as well as its concentration. NMR spectroscopy confirms that the silicon of the chain transfer agent is incorporated into the polymer. The stability of the catalyst toward polar monomer enables the chain transfer polymerization of semi-telechelic poly(ethylene-methyl acrylate) copolymers.


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