The patent badge is an abbreviated version of the USPTO patent document. The patent badge does contain a link to the full patent document.

The patent badge is an abbreviated version of the USPTO patent document. The patent badge covers the following: Patent number, Date patent was issued, Date patent was filed, Title of the patent, Applicant, Inventor, Assignee, Attorney firm, Primary examiner, Assistant examiner, CPCs, and Abstract. The patent badge does contain a link to the full patent document (in Adobe Acrobat format, aka pdf). To download or print any patent click here.

Date of Patent:
Apr. 09, 2019

Filed:

Jul. 31, 2015
Applicant:

Nanjing University of Technology, Nanjing, Jiangsu Province, CN;

Inventors:

Weihong Xing, Nanjing, CN;

Honglin Mao, Nanjing, CN;

Rizhi Chen, Nanjing, CN;

Hongnian Shang, Nanjing, CN;

Nanping Xu, Nanjing, CN;

Attorney:
Primary Examiner:
Int. Cl.
CPC ...
C07C 249/04 (2006.01); C07C 251/44 (2006.01); B01J 29/89 (2006.01); C07C 251/38 (2006.01);
U.S. Cl.
CPC ...
C07C 249/04 (2013.01); B01J 29/89 (2013.01); C07C 251/38 (2013.01); C07C 251/44 (2013.01);
Abstract

The invention relates to a solvent-free green ammoximation process based on membrane distribution with a procedure as: adding TS-1 catalyst and ketone into a reactor in advance; setting the stirring speed and reaction temperature; after reaching the set temperature, adding a certain amount of ammonia and hydrogen peroxide into a reaction solution, wherein the hydrogen peroxide is fed in a way of using membrane as a distributor, the ammonia is fed in a continuous or semi-continuous manner; oxime is produced upon the reaction. The advantages of the invention include the mild reaction conditions, high reacting efficiency, simple operation and environmentally-friendly process. And there is no need to add any solvent during the reaction process. During the ammoximation reaction, both the conversion rate of the ketone and the selectivity of the oxime can be over 98.0%.


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