The patent badge is an abbreviated version of the USPTO patent document. The patent badge does contain a link to the full patent document.

The patent badge is an abbreviated version of the USPTO patent document. The patent badge covers the following: Patent number, Date patent was issued, Date patent was filed, Title of the patent, Applicant, Inventor, Assignee, Attorney firm, Primary examiner, Assistant examiner, CPCs, and Abstract. The patent badge does contain a link to the full patent document (in Adobe Acrobat format, aka pdf). To download or print any patent click here.

Date of Patent:
Oct. 02, 2018

Filed:

Oct. 23, 2015
Applicant:

Tetraphase Pharmaceuticals, Inc., Watertown, MA (US);

Inventors:

Wu-Yan Zhang, Lexington, MA (US);

Danny LaFrance, Natick, MA (US);

Magnus P. Ronn, Melrose, MA (US);

Assignee:

Tetraphase Pharmaceuticals, Inc., Watertown, MA (US);

Attorney:
Primary Examiner:
Int. Cl.
CPC ...
C07D 295/15 (2006.01); C07C 231/12 (2006.01); C07C 245/20 (2006.01); C07C 237/26 (2006.01);
U.S. Cl.
CPC ...
C07D 295/15 (2013.01); C07C 231/12 (2013.01); C07C 237/26 (2013.01); C07C 245/20 (2013.01); C07C 2603/46 (2017.05);
Abstract

Provided herein are improved processes for convening C7-amino-substituted tetracylines to C7-fluoro-substituted tetracyclines as well as intermediates produced by or used in these processes. In one embodiment, a thermal fluorination method is provided in which a suspension comprising a non-polar organic solvent and a C7-diazo-substituted tetracycline hexafluorophosphate, hexafluoarsenate or hexafluorosilicate salt, or a salt, solvate or combination thereof, is healed to provide a C7-fluoro-substituted tetracyline, or salt, solvate or combination thereof. In another embodiment, a photolytic fluorination is provided in which a solution comprising an ionic liquid and a C-7diazo-substituted tetracyline tetrafluoroborate, hexafluorophosphate, hexafluoroarsenate or hexafluorosilicate salt, or a salt, solvate or combination thereof, is irradiated to provide a C7-fluoro-substituted tetracyline, or salt, solvate or combination thereof.


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