Harvard College

University System of Maryland

North Carolina State University

The Mitre Corporation

Ronald Lee Walsworth

Matthew James Turner

Linh My Pham

David Glenn

Matthew Scot Rosen

Mikhail D Lukin

John Francis Barry

Chinmay Belthangady

Nir Bar-Gill

Jennifer May Schloss

Dominik Bucher

Nithya Arunkumar

Stephen J Devience

Connor A Hart

Hongkun Park

Marko Loncar

Jacob M Taylor

Jeff Lichtman

Amir Yacoby

Narayanan Kasthuri

Richard Schalek

Liang Jiang

Thomas Theis

Igor Lovchinsky

Lilian I Childress

Daniel T Walters

Mikael Paul Backlund

Nicholas Ryan Langellier

Alexander Sushkov

Pauli Kehayias

Nicholas Chisholm

Huiliang Zhang

Erik Bauch

David Lesage

Paola Cappellaro

Edlyn Victoria Levine

David Le Sage

Systems and methods of quantum sensing include depositing a sample volume onto an ensemble of quantum defects, hyperpolarizing spins in the sample volume, performing a sensing sequence, and reading out information regarding electronic spin states of the quantum defects in the ensemble of quantum defects, which sense the hyperpolarized spins in the sample volume.

Systems and methods for quantum sensing with signal amplification by reversible exchange

Systems and methods of quantum sensing include obtaining information regarding a target signal in electronic spin states of quantum defects in an ensemble of quantum defects, mapping the information regarding the target signal from the electronic spin states of the quantum defects to corresponding nuclear spin states associated with the quantum defects, applying a light pulse to the ensemble of quantum defects to reset the electronic spin states of the quantum defects, and repeating a readout stage a plurality of times within a readout duration. The readout stage includes mapping the information regarding the target signal back from the nuclear spin states to the corresponding electronic spin states and applying a data acquisition readout pulse to optically measure the electronic spin states of the quantum defects.

Systems and methods for quantum sensing using solid-state spin ensembles

Devices for determining a state of a magnetic field-generating article are provided. In various embodiments, a device comprises: a single crystal diamond having a plurality of NV centers, the single crystal diamond configured to be disposed adjacent to a magnetic field-generating article, and configured to generate a fluorescent signal in response to being illuminated by a light source; a coherent light source configured to generate a light beam directed at the single crystal diamond; a microwave (MW) radiation source configured to irradiate the single crystal diamond with a MW signal; a magnetic field source configured to apply a bias magnetic field to the single crystal diamond; a photosensor configured to collect the fluorescent signal generated by the single crystal diamond; and a computing node operatively coupled to each of the coherent light source, the MW radiation source, the magnetic field source, and the photosensor.

High-resolution magnetic field fingerprinting of integrated circuit activity with a quantum diamond microscope

A method and system of measuring a direct current magnetic field using a plurality of spin centers are disclosed. A spin bath associated with the spin centers may be driven with a first source of electromagnetic radiation to reduce dephasing of the spin centers. The spin centers may be measured using double quantum (DQ) magnetometry in order to reduce the effects of crystal strain on spin dephasing times. An electromagnetic response of at least one of the plurality of spin centers may be observed using an electromagnetic radiation collection device. Accordingly, up to an eight times improvement in DC field sensitivity may be accomplished for a spin center ensemble.

Control and cancellation of spin bath induced dephasing in solid-state ensembles

Solid-state spin sensor systems and methods of manufacturing are disclosed. A mounting structure may be provided in thermal contact with a solid-state spin sensor having a plurality of color center defects such that thermal energy flows from the solid-state spin sensor to the mounting structure. A microwave application structure may be disposed on a face of the mounting structure or a face of the solid-state spin sensor for applying microwave radiation to the solid-state spin sensor.

Integrated mounting solution for solid-state spin sensors used for bulk detection and imaging

A synchronized readout (SR) technique for spectrally selective detection of oscillating magnetic fields with sub-millihertz resolution, using coherent manipulation of solid state spins.

Synchronized-readout for narrowband detection of time-varying electromagnetic fields using solid state spins

A system and method for performing vector magnetometry are described. A method can include illuminating diamond with a modulated optical signal and a modulated microwave (MW) signal. A first, bias magnetic field is also applied to the diamond. Light emitted from the diamond in response to the optical signal, the MW signal, and the first magnetic field is detected via a single detector at a fixed position relative to the diamond. A modulation of the detected light encodes information corresponding to a plurality of nitrogen vacancy (NV) axes of the diamond.

Simultaneous vector magnetometry with nitrogen vacancy centers in diamond or other solid-state spin sensors

Methods and systems for Nuclear Magnetic Resonance (NMR) spectra of samples having unresolved peaks are described. The methods and systems allow for the creation nuclear spin singlet states in nearly-equivalent spin pairs, for example, using continuous spin-locking with a nutation frequency matched to the coupling strength between spins. The invention relates generally to the field Nuclear Magnetic Resonance (NMR). Nuclear magnetic resonance (NMR) spectroscopy can be used as a tool for determining the chemical structure and/or geometry of a molecule in a sample. In many samples, however, resonance frequencies of different nuclei fully or partially overlap, which makes chemical identification of molecule(s) in a sample difficult or impossible.

Creation of nearly-equivalent nuclear spin singlet states using spin-lock induced crossing

A solid state electronic spin system contains electronic spins disposed within a solid state lattice and coupled to an electronic spin bath and a nuclear spin bath, where the electronic spin bath composed of electronic spin impurities and the nuclear spin bath composed of nuclear spin impurities. The concentration of nuclear spin impurities in the nuclear spin bath is controlled to a value chosen so as to allow the nuclear spin impurities to effect a suppression of spin fluctuations and spin decoherence caused by the electronic spin bath. Sensing devices such as magnetic field detectors can exploit such a spin bath suppression effect, by applying optical radiation to the electronic spins for initialization and readout, and applying RF pulses to dynamically decouple the electronic spins from the electronic spin bath and the nuclear spin bath.

Use of nuclear spin impurities to suppress electronic spin fluctuations and decoherence in composite solid-state spin systems

Systems and methods for magnetic sensing and imaging include a sensor having a network of isolated electron-spin quantum bits (qubits) disposed on the surface of the sensor; and a solid state electronic spin system disposed below the surface of the sensor, wherein the solid state electronic spin system has a spin-state dependent fluorescence; a source of light; a source of first external perturbation, wherein the source of first external perturbation generates a magnetic field; a source of second external perturbation; wherein, the source of light and the first and second external perturbations are configured to coherently and independently manipulate the spin states of at least one qubit and at least one solid state electronic spin system; and a detector to optically measure the solid-state electronic spins spin-state dependent fluorescence.

Magnetic sensing and imaging using interactions between surface electron spins and solid state spins

Methods and systems for Nuclear Magnetic Resonance (NMR) spectra of complex chemical mixtures are described. The methods and systems allow undesired NMR spectral background to be removed or suppressed and target spectral peaks to be uncovered, for example, when strong background signals overlap weaker peaks. In some embodiments, the methods and systems employ a quantum filter utilizing nuclear spin singlet states.

Nuclear singlet states as a contrast mechanism for NMR spectroscopy

Long spin coherence lifetimes are realized for ensembles of electronic spin impurities in solid state spin systems, for example NV color centers in diamond, by using spin-control RF pulse sequences to provide dynamic decoupling of the ensembles of spin impurities from environmental sources of decoherence such as dipolar and hyperfine interactions with proximal spin and other paramagnetic impurities in diamond. In this way, the measurement sensitivity of the coherent evolution of ensembles of solid state spin impurities are increased. Using the Carr-Purcell-Meiboom-Gill (CPMG) pulse sequence, the spin coherence lifetimes of NV ensembles can be extended to more than 2 ms in room temperature diamond, and sensitivity of magnetometry that uses NV ensembles can be increased.

Dynamic decoupling in solid state spin ensembles

Absorption based detection of spin states of spin impurities within a solid-state spin system, such as NV centers in diamond, is implemented by measuring the absorption intensity of an optical signal applied to the spin impurities, i.e. change in intensity of the optical signal after the signal has been transmitted through the solid-state spin system. During optical excitation of the spin impurities, microwave pulses are applied to the sample at a frequency tuned to the ESR frequency. The relative populations of the spin states of the impurities, which provides information regarding variables of interest such as an external magnetic field or a quantum information protocol, is determined from the ratio of the absorption intensity of the optical signal when the microwave pulses are turned on, to the absorption intensity of the optical signal when the microwave pulses turned off.

Absorbtion-based detection of spin impurities in solid-state spin systems

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Newton, MA, United States of America

Ronald Lee Walsworth