Princeton University

International Business Machines Corporation

William Marsh Rice University

Corning Incorporated

The Science and Technology Facilities Council

United Kingdom Research and Innovation

Gerard Wysocki

William M Green

Eric J Zhang

Frank K Tittel

Chu Cheyenne Teng

Jonas Westberg

Chi Xiong

Yin Wang

Stephen So

J Patrick Frantz

Chu C Teng

Lukasz Sterczewski

Cheyenne Teng

Michal Nikodem

Chung-En Zah

Feng Xie

Damien Weidmann

Robert F Curl

Matthias Dittberner

Genevieve Plant

Yifeng Chen

Andreas Hangauer

According to various embodiments, a system for stabilizing operation of semiconductor laser frequency combs via optical feedback is disclosed. The system includes an external cavity having a beam-splitter, polarizer, and mirror or partially reflective element mounted on a translational stage. The external cavity and a laser facet of the semiconductor laser form an external optical resonator for coupling light to a laser cavity.

System and method for optical feedback stabilized semiconductor frequency combs

Disclosed are a system and method for active stabilization of parasitic fringes in optical spectrometers, wherein the spectrometer obtains the transmission spectrum, and a signal processor extracts the etalon drift from the spectral signatures of parasitic fringes. The disclosed approach improves spectrometer accuracy, minimizes drift, and increases time between calibrations.

Active stabilization of parasitic fringes in optical spectrometers

Disclosed herein is an all-digital phase and timing correction procedure for coherent averaging in dual-comb and multiheterodyne spectroscopy&#x2014;applicable to any dual-comb spectroscopy setup. It can account for large frequency/phase instabilities of the used sources, yielding a significant reduction of the noise pedestal and an increase in signal-to-noise ratio (SNR) of the radio frequency (RF) beat notes. This technique is computationally efficient and can be conveniently implemented either as a post-processing algorithm or in a real-time data acquisition and processing platform without the necessity of adding any additional optical elements to the dual-comb spectroscopy system. By implementing this technique, the performance of any comb- or comb-like-source-based DCS system with a sufficient degree of mutual coherence between the optical modes can be improved in terms of SNR and number of spectroscopically-usable RF beat notes. The described technique is compatible with a DC-centered RF spectrum, where the negative frequencies are folded to the positive domain to double the number of beat notes within the detector bandwidth. The technique enables coherent averaging over extended time-scales even for free-running combs, thus increasing the sensitivity of absorption and dispersion DCS measurements.

Fast computational phase and timing correction for multiheterodyne spectroscopy

A method is provided for Fourier domain dynamic correction of optical fringes in a laser spectrometer. The method includes Fourier transforming a background spectrum contaminated with the optical fringes to obtain baseline fringes in a frequency domain. The method includes partitioning the baseline fringes in the frequency domain to obtain partitioned baseline fringes. The method includes reconstructing the partitioned baseline fringes as separate spectra. The method includes constructing a fitting model to approximate the background spectrum by assigning a first and a second free parameter to each of partitioned baseline fringe components to respectively allow for drift and amplitude adjustments during a fitting of the fitting model. The method includes applying the fitting model to a newly acquired spectrum to provide an interpretation of the newly acquired spectrum having a reduced influence of spectral contamination on concentration retrieval.

Fourier domain dynamic correction method for complex optical fringes in laser spectrometers

A generalized feed-forward method for accurate tunable laser absorption spectroscopy includes generating a laser beam. The generated laser beam is directed down a reference path and a test/sample path. One or more parameters are extracted from the reference path. The one or more parameters, extracted from the reference path, are used as feed-forward, to adjust spectral analysis of the test/sample path to detect a composition and/or concentration of an analyte gas within the test/sample path. The extraction of the one or more parameters from the reference path and the spectral analysis of the test/sample path are performed substantially concurrently.

Feed-forward spectral calibration methodology for line-scanned tunable laser absorption spectroscopy

An on-chip spectroscopic sensor includes a tunable diode laser. A laser driver for drives the tunable diode laser. An analyte test cavity receives a chemical sample and exposes the received chemical sample to light from the tunable diode laser. An optical detector detects light emerging from the analyte test cavity as a result of the laser exposure. A spectral analyzer determines a spectrum of the emerging light, matches and removes one or more known optical fringe patterns from the determined spectrum, and determines a composition or concentration of the chemical sample from the optical fringe pattern-removed spectrum.

On-chip spectroscopic sensors with optical fringe suppression

A tunable diode laser absorption spectroscopy device includes a tunable diode laser. A laser driver is configured to drive the diode laser and ramp it within a particular frequency range. An analyte gas container, a reference gas container, and a fringe generating device are configured to receive the laser therethrough. An optical detector is configured to detect the laser after it has passed through the analyte gas container and/or the reference gas container, and the in-line fringe generating device. An acquisition card is configured to sample an output of the optical detector. A spectral analyzer is configured to receive output data from the acquisition card, determine a spectrum of the output data, decouple the fringe spectrum from the measured spectrum, calibrate the spectrum based on an expected ideal spectrum of both the fringe and reference gas, and determine a composition of the analyte based on the calibrated spectrum.

Tunable diode laser absorption spectroscopy with corrected laser ramping nonlinearities

A sensitivity boosted laser dispersion spectroscopy system for sensing a sample in a sample cell or in an open path crossing the sample. The system includes a local oscillator arm and a sample arm containing the sample cell or the open path crossing the sample. A laser source is configured to generate a first light beam directed along the sample arm and a second light beam, the second light beam being frequency shifted and directed along the local oscillator arm. An intensity modulator/phase modulator/frequency shifter is disposed in the sample arm configured to generate a multi-frequency beam having known frequency spacing which is then passed through the sample cell to generate a sample arm output. A beam combiner is configured to combine the sample arm output and the second light beam from the local oscillator arm and generate a combined beam. A photodetector is configured to detect the combined beam for sensing the sample in the sample cell.

Chirped laser dispersion spectroscopy sensitivity booster

A method is provided for Fourier domain dynamic correction of optical fringes in a laser spectrometer. The method includes Fourier transforming a background spectrum contaminated with the optical fringes to obtain baseline fringes in a frequency domain. The method includes partitioning the baseline fringes in the frequency domain using bandpass filtering to obtain partitioned baseline fringes. The method includes reconstructing the partitioned baseline fringes as separate spectra using an inverse Fourier transform. The method includes constructing a fitting model to approximate the background spectrum by assigning a first and a second free parameter to each of partitioned baseline fringe components to respectively allow for drift and amplitude adjustments during a fitting of the fitting model. The method includes applying the fitting model to a newly acquired spectrum to provide an interpretation of the newly acquired spectrum having a reduced influence of spectral contamination on concentration retrieval.

A system for simultaneous optical pathlength determination and remote chemical sensing of a sample disposed along an optical path. A modulated laser source configured for modulated light emission so that at least one spectral sideband with a sideband frequency is created, the modulated light emission is directed along the optical path and sideband frequency is varied over time. A detector is configured to detect transmitted light along the optical path and generate a detected light intensity signal. A frequency down-converter is configured to receive the detected light emission signal and generate a frequency down-converted light intensity signal. A demodulator is configured to demodulate the frequency of the down-converted light intensity signal and output an instantaneous frequency. A pathlength calculator is configured to determine an optical pathlength to the sample based on the instantaneous frequency. A frequency down-converted light intensity signal is simultaneously output for spectroscopic chemical sensing.

Simultaneous ranging and remote chemical sensing utilizing optical dispersion or absorption spectroscopy

Method and apparatus for detecting a species in a dilute medium, the species having a spectral feature, the apparatus comprising: a beam source arranged to generate a first laser beam and a second laser beam coherent with each other, and having a matching chirp pattern. Beam guide arranged to pass at least the first laser beam through the dilute medium; a beam mixer arranged to mix the first and the second laser beams to form a mixed beam. Detector arranged to detect, during the chirp pattern, the mixed beam and to measure changes in the mixed beam caused by refractive index variations in the dilute medium across a spectral feature. Output providing a signal that changes in response to the measured changes.

Detecting species in a dilute medium

An apparatus and method for differential optical dispersion using a first sample and a second sample are disclosed. The apparatus includes a single frequency chirped laser source configured to generate a single frequency chirped laser beam. A first beam splitter is configured to split the single frequency chirped laser beam into first and second optical branches, the first sample being located in the first optical branch, the second sample being located in the second optical branch. A frequency shifter is located in the second optical branch, downstream of the second sample. A second beam splitter is configured to combine the first and second optical branches and generate a chirp-modulated mixed light beam. A square law detector is configured to detect the chirp-modulated mixed light beam and generate a heterodyne beatnote signal. A demodulator is configured for detection of the heterodyne beatnote signal to generate a transmission/differential optical dispersion spectrum.

Optical subtraction of molecular dispersion signals enabled by differential optical dispersion spectroscopy

An apparatus and method for detecting refractive index variations in a sample is disclosed. The apparatus includes a multi frequency laser source configured to generate a mixed laser beam having at least two optical frequencies. A sinusoidal function generator is configured to modulate the optical frequencies to generate a chirp-modulated mixed laser beam. The chirp-modulated mixed laser beam being configured to pass through the sample. A detector is configured to detect the chirp-modulated mixed beam. A signal processer is configured to process the detected chirp-modulated mixed beam to measure refractive index variations in the sample.

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Princeton, NJ, United States of America

Gerard Wysocki